There is no best place Sigils as they drop everywhere. I have so many Sigils that I though they grow on trees. They are the most common drops among all the reagents. You'll get so many of them that you will really wished you get something else.
Anyway, last map area, anywhere after Mead River, I think.
Moonbug
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Anyway, last map area, anywhere after Mead River, I think.